聚环氧乙烷基电解质结构设计与离子传输机制研究进展

郑肖杰; 俞尚长; 何奇霖; 董盼盼; 杨维清

doi:10.19799/j.cnki.2095-4239.2026.0372

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聚环氧乙烷基电解质结构设计与离子传输机制研究进展

更新时间：2026-06-03

- 聚环氧乙烷基电解质结构设计与离子传输机制研究进展
- Progress in Structural Design and Ion Transport Mechanisms of PEO-Based Electrolytes
- 储能科学与技术 2026年页码：1-22
- 作者机构：
  
  1.西南交通大学，化学学院，四川成都 610031
  2.西南交通大学，材料先进技术教育部重点
  3.实验室，材料科学与工程学院，四川成都 610031，西南交通大学，前沿科学研究院，四川;;成都 610031）;图片摘要
- 作者简介：
- 基金信息：
- DOI：10.19799/j.cnki.2095-4239.2026.0372
  中图分类号： TK 02
- 网络首发：2026-06-03，
- 稿件说明：
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郑肖杰, 俞尚长, 何奇霖, 等. 聚环氧乙烷基电解质结构设计与离子传输机制研究进展[J/OL]. 储能科学与技术, 2026,1-22.

ZHENG Xiaojie, YU Shangchang, HE Qinlin, et al. Progress in Structural Design and Ion Transport Mechanisms of PEO-Based Electrolytes[J/OL]. Energy Storage Science and Technology, 2026, 1-22.
郑肖杰, 俞尚长, 何奇霖, 等. 聚环氧乙烷基电解质结构设计与离子传输机制研究进展[J/OL]. 储能科学与技术, 2026,1-22. DOI： 10.19799/j.cnki.2095-4239.2026.0372.

ZHENG Xiaojie, YU Shangchang, HE Qinlin, et al. Progress in Structural Design and Ion Transport Mechanisms of PEO-Based Electrolytes[J/OL]. Energy Storage Science and Technology, 2026, 1-22. DOI： 10.19799/j.cnki.2095-4239.2026.0372.

摘要

针对聚环氧乙烷（PEO）基固态电解质中离子电导率、机械强度与界面稳定性难以兼顾的核心瓶颈及其突破策略，本文从聚合物本体结构设计出发，介绍了四种改性方法：深共晶溶剂原位增塑，通过与PEO链段竞争配位Li

，弱化Li

与醚氧相互作用，提升离子电导率与锂离子迁移数；离子液体封装于交联网络，构建聚合物与离子液体双重传导路径，增强界面稳定性；硫醇-烯点击化学构建半互穿网络，引入短链增塑剂降低链段运动能垒，并采用双盐体系原位构筑富LiF界面层；热压层合制备锂化有机纳米纤维增强网络，利用氢键与界面快速传输通道协同提升离子电导率与力学性能。在复合电解质设计中，阐述了三种协同增强策略：金属有机框架中开放金属位点对TFSI

的强配位固定，促进锂盐解离并提高锂离子迁移数；热塑性聚氨酯与二维锂镁硅酸盐纳米片的复合，通过Lewis酸位点固定阴离子并抑制PEO结晶；Janus层调控LLZTO/PEO界面化学相容性，同时解决填料团聚、阴离子迁移及界面副反应。针对硅碳负极界面，提出了预浸润处理构建连续聚合物离子传导网络，显著提升活性材料利用率与循环稳定性。本研究系统揭示了PEO基电解质中离子传输的多尺度调控机制，为高比能全固态锂金属电池的理性设计提供了实验依据与理论支撑，并对复合聚合物电解质的产业化发展方向进行了展望。

Abstract

Poly(ethylene oxide) (PEO)-based solid-state electrolytes face a long-standing trade-off among ionic conductivity

mechanical strength

and interfacial stability. This study summarizes recent progress in breaking this bottleneck through structural design and ion transport mech

anism modulation of PEO-based electrolytes. For polymer bulk structure design

we introduce four modification methods: (i) in situ formation of deep eutectic solvents weakens Li

-ether oxygen coordination via competitive binding

significantly increasing ionic conductivity and Li

ion transference number; (ii) encapsulation of ionic liquids in cross-linked networks constructs dual polymer and ionic liquid conduction pathways and enhances interfacial stability; (iii) thiol-ene click chemistry builds a semi-interpenetrating network with short-chain plasticizers to lower chain motion energy barriers

and a dual-salt system in situ forms a LiF-rich interface layer; (iv) thermal lamination produces lithiated organic nanofiber-reinforced composite electrolytes

where hydrogen bonding and interfacial fast-transport channels synergistically improve ionic conductivity and mechanical strength. Regarding composite electrolyte design

we elaborate three synergistic strategies: (i) exposed metal sites in metal-organic frameworks strongly anchor TFSI

promoting lithium salt dissociation and raising Li

ion transference number; (ii) thermoplastic polyurethane combined with two-dimensional lithium magnesium silicate nanosheets uses Lewis acid sites to fix anions and suppress PEO crystallization; (iii) a Janus layer regulates chemical compatibility at the LLZTO/PEO interface

resolving filler agglomeration

anion migration

and interfacial side reactions. To address the silicon-carbon anode interface

we propose a pre-infiltration treatment that builds a continuous polymer ion conduction network

markedly improving active material utilization and cycling stability. Collectively

these studies systematically reveal multi-scale ion transport regulation mechanisms in PEO-based electrolytes

providing experimental evidence and theoretical support for rational design of high-specific-energy all-solid-state lithium metal batteries. Finally

we prospect the industrial development direction of

composite polymer electrolytes.

关键词

Keywords

references

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